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1 article(s) from Sundermann, Uschi

Quantification of N-acetylcysteamine activated methylmalonate incorporation into polyketide biosynthesis

Stephan Klopries,
Uschi Sundermann and
Frank Schulz

Beilstein J. Org. Chem. 2013, 9, 664–674, doi:10.3762/bjoc.9.75

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Figure 1: The most intensively studied PKS, deoxyerythronolide B synthase (DEBS), which catalyzes the key ste...

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Scheme 1: Synthesis of SNAC-activated D₃-methylmalonate. a: 2.1 equiv [(CH₃)₂CH]₂NLi, 1 equiv CD₃I, abs. THF,...

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Figure 2: Structures of erythromycin (left) and rapamycin (right). In this experiment both compounds were lab...

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Figure 3: Relative incorporation of the D₃-label into erythromycin (A) and rapamycin (B), depending on the fe...

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Figure 4: ESI–MS spectra of feeding experiments with an erythromycin-producing culture of S. erythraea. The m...

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Scheme 2: Incorporation of a propargylated malonic acid derivative into erythromycin through an active-site m...

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Published 05 Apr 2013

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